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b(the)f(rep)q(orted)g fe(\013)p fm(-particle)h (energies)-47 1446 y(probably)d(do)f(not)h(b)q(elong)g(to)g(branc)o(hes)f(to) g(the)g(ground-states)h(of)f(their)h(daugh)o(ters,)f(they)f(nev)o(ertheless) -47 1506 y(giv)o(e)g(information)i(of)f(use)f(for)h(getting)g(go)q(o)q(d)h (estimates)f(of)f(the)g(masses)h(for)f(v)o(ery)f(hea)o(vy)h(n)o(uclides.)-47 1602 y(Another)h(imp)q(ortan)o(t)i(disco)o(v)o(ery)d(in)i(this)h(region)f(is) h(due)e(to)h(a)g(collab)q(oration)j(of)c(Liv)o(ermore)h(and)g(Dubna)-47 1662 y(who)i(found)f(the)g(existence)g(of)g(a)h(sub-shell)h(closure)f(at)f fe(N)5 b fm(=162.)32 b(In)19 b(a)g(\014rst)h(pap)q(er)g(they)e(rep)q(orted)i (the)-47 1722 y(observ)m(ation)f(of)f(t)o(w)o(o)f(new)g(isotop)q(es)i(of)f (elemen)o(t)e fe(Z)t fm(=106)j(and)f(in)o(terpreted)f(the)g(results)h(as)g (evidence)e(for)-47 1782 y(extra)g(stabilit)o(y)j(at)e fe(Z)t fm(=108)h(and)f fe(N)5 b fm(=162)19 b([94Laza)q(].)k(And)16 b(at)h(this)h(ENAM'95)e(conference,)g(Oganessian)-47 1842 y(et)h(al.)27 b([95Ogan)q(])17 b(rep)q(orted)h(the)g(disco)o(v)o(ery)f(of)850 1824 y fi(273)905 1842 y fm(Xa,)g(the)h(\014rst)g(n)o(uclide)g(with)h fe(N)5 b fm(=163,)19 b(whic)o(h)f(exhibits)-47 1903 y(a)f(strong)h(increase)g (of)f(the)g fe(\013)p fm(-energy)l(,)g(strongly)h(indicating)i(the)d (subshell)h(closure)g(at)f fe(N)5 b fm(=162.)25 b(Suc)o(h)17 b(an)-47 1963 y(e\013ect)d(could)i(b)q(e)f(resp)q(onsible)i(for)e(the)f (amazing)j(fact)d(that)i(the)e(increasing)j(probabilit)o(y)g(for)e(sp)q(on)o (taneous)-47 2023 y(\014ssion,)21 b(so)f(eviden)o(t)f(for)h(elemen)o(ts)f(un) o(til)h fe(Z)t fm(=104,)h(is)g(far)f(less)g(prominen)o(t)g(than)g(exp)q (ected)e(b)q(ey)o(ond)i(the)-47 2083 y(latter)f(elemen)o(t.)29 b(One)19 b(of)h(us)f([95W)l(aps)r(])f(plans)j(to)e(publish)i(an)f(analysis)h (of)f(some)f(of)h(these)f(p)q(oin)o(ts)h(and)-47 2143 y(the)f(ones)h (discussed)h(b)q(elo)o(w)g(\(section)f(5.4\).)32 b(It)19 b(is)h(also)i(in)o (teresting)e(to)g(note)g(that,)h(in)f(a)g(recen)o(t)e(pap)q(er,)-47 2204 y(Brenner)13 b(et)h(al.)22 b(found,)15 b(in)g(an)g(analysis)i(of)e(the)f (\014rst)h(2)976 2186 y fi(+)1020 2204 y fm(states)g(in)g(ev)o(en-ev)o(en)e (n)o(uclides,)i(that)g(a)f(spherical)-47 2264 y(subshell)20 b(migh)o(t)f(close)g(at)g fe(N)5 b fm(=164)20 b([95Bren)o(].)28 b(It)18 b(w)o(ould)i(b)q(e)f(in)o(teresting)g(to)g(rep)q(eat)g(this)g (analysis)i(with)-47 2324 y(the)16 b(assumption)i(of)e(a)h(sub-shell)h (closure)f(at)f fe(N)5 b fm(=162)18 b(as)f(observ)o(ed)f(b)o(y)f([95Ogan)r (].)-47 2526 y ff(4.)37 b(New)26 b(data)i(from)c(mass)g(sp)r(ectrom)o(etry) -47 2650 y fl(4.1.)31 b(Stable)23 b(n)n(uclides)-47 2778 y fm(Data)14 b(with)g(high)g(precision)h(\(of)e(the)g(order)g(of)h(1)f(part)h (in)f(10)1055 2760 y fi(10)1094 2778 y fm(\))g(are)g(rep)q(orted)g(b)o(y)g (the)g(MIT)f(group)j([94DiFi)q(])-47 2838 y(using)j(a)f(P)o(enning-trap)h(sp) q(ectrometer.)23 b(A)16 b(careful)h(ev)m(aluation)i(of)e(the)g(systematic)g (errors)g(and)g(analysis)-47 2898 y(of)d(the)f(obtained)j(data)e(allo)o(w)o (ed)h(this)g(group)g(to)f(ac)o(hiev)o(e)f(v)o(ery)f(satisfactory)k(in)o (ternal)e(consistency)h(c)o(hec)o(ks.)p eop %%Page: 3 3 bop -47 30 a fm(Their)18 b(impressiv)o(e)g(rep)q(ort)g([94DiFi)r(])f(is,)h (in)h(this)f(sense,)g(recommendably)g(complete.)25 b(Y)l(et,)17 b(they)g(should)-47 90 y(not)i(remain)g(unc)o(hallenged:)27 b(c)o(hec)o(ks)17 b(b)o(y)h(another)h(group,)h(at)f(the)f(same)h(lev)o(el)g (of)f(precision,)j(are)d(highly)-47 150 y(desirable)24 b(to)g(strengthen)g (the)f(v)m(alidit)o(y)i(of)f(their)g(mass)g(measuremen)o(ts,)g(and)g (transform)g(these)f(v)o(ery)-47 210 y(precise)17 b(measuremen)o(ts)g(in)o (to)i(v)o(ery)d(accurate)i(ones.)26 b(Some)18 b(of)g(their)g(results)h(w)o (ere)e(already)h(used)g(in)h(the)-47 271 y(1993)c(tables)f(and)h(ha)o(v)o(e)d (b)q(een)i(revised)f(only)i(sligh)o(tly)g(\(except)d(for)i(the)1274 252 y fi(12)1311 271 y fm(C+)1384 252 y fi(2)1404 271 y fm(H{)1465 252 y fi(14)1502 271 y fm(N)f(com)o(bination\).)22 b(New)-47 331 y(is)d(the)f(result)i(for)305 313 y fi(28)343 331 y fm(Si)f(where)f(2)h (orders)g(of)g(magnitude)h(in)f(precision)h(ha)o(v)o(e)d(b)q(een)i(gained)h (compared)e(to)-47 391 y(AME-93.)29 b(F)l(rom)19 b(this)g(result)h(follo)o(w) g(impro)o(v)o(ed)e(v)m(alues)i(for)f(the)g(other)f(stable)i(Si)g(isotop)q (es.)30 b(This)20 b(ma)o(y)-47 451 y(b)q(ecome)15 b(imp)q(ortan)o(t)i(in)f (future)f(for)h(the)g(de\014nition)h(of)f(the)f(mass)h(unit,)g(the)g(kg.)21 b(If)15 b(it)h(is)g(de\014ned)g(in)g(terms)-47 511 y(of)j(the)g(atomic)h (mass)f(unit,)h(b)o(y)f(accepting)h(a)f(de\014ned)g(v)m(alue)h(for)f(the)g (Av)o(ogadro)h(constan)o(t,)f(realization)-47 571 y(of)e(a)g(mass)g(standard) h(ma)o(y)e(b)q(e)h(b)q(est)g(done)f(b)o(y)h(constructing)g(an)g(ultrapure)h (Si)f(crystal.)23 b(New)16 b(also)i(is)g(the)-47 632 y(result)f(for)163 614 y fi(15)200 632 y fm(N,)f(of)g(imp)q(ortance)h(for)g(the)f(calibration)j (of)d fe(\015)s fm(-ra)o(y)h(energies)f(\(see)g(section)h(5.1\).)-47 727 y(Other)f(groups)h(w)o(orking)h(with)f(P)o(enning-trap)h(sp)q (ectrometers)e(in)h(Ohio)g(and)g(Sto)q(c)o(kholm)g(ha)o(v)o(e)e(obtained)-47 787 y(results)24 b(for)g(D,)271 769 y fi(20)309 787 y fm(Ne,)406 769 y fi(22)443 787 y fm(Ne)f(and)627 769 y fi(28)664 787 y fm(Si)i(\(and)f(a)g(preliminary)g(v)m(alue)h(for)e(the)h(h)o(ydrogen)f (mass\))h(whic)o(h)-47 848 y(con\014rm,)14 b(at)g(their)g(resp)q(ectiv)o(e)f (lev)o(el)h(of)h(accuracies,)f(the)g(corresp)q(onding)i(more)d(precisely)h (kno)o(wn)h(masses.)-47 943 y(Classical)24 b(mass-sp)q(ectrometry)d(on)h (stable)g(and)g(nearly)g fe(\014)s fm(-stable)g(n)o(uclides)f(along)j(the)d (\\bac)o(kb)q(one")h(is)-47 1003 y(also)c(pro)q(ducing)h(results,)e(lik)o(e)g (the)g(new)f(v)m(alues)i(for)f(Xe,)f(obtained)i(at)g(Winnip)q(eg.)24 b(Their)18 b(planned)g(mea-)-47 1064 y(suremen)o(ts)c(on)i(Hg)f(isotop)q(es)i (to)e(solv)o(e)h(the)f(mercury)f(problem)h(\(section)h(7)g(in)f([IV)o(]\))g (are)g(eagerly)g(a)o(w)o(aited.)-47 1268 y fl(4.2.)31 b(Nuclides)23 b(far)g(from)f(stabilit)n(y)-47 1396 y fm(The)c(regions)h(somewhat)g(remo)o (v)o(ed)e(from)h(the)g(line)h(of)f(stabilit)o(y)l(,)i(esp)q(ecially)g(the)e (most)g(exotic)g(n)o(uclides,)-47 1456 y(are)13 b(of)g(in)o(terest)g(in)h (helping)h(to)e(determine)g(the)g(y)o(et)f(p)q(o)q(orly)j(kno)o(wn)e(b)q(eha) o(vior)h(of)g(the)f(binding)i(energies)e(for)-47 1516 y(large)f (di\013erences)g(b)q(et)o(w)o(een)f(n)o(um)o(b)q(ers)g(of)h(neutrons)h(and)f (of)g(protons.)21 b(This)13 b(is)f(re\015ected)f(in)h(the)f(excessiv)o(ely) -47 1577 y(large)17 b(deviations)h(amongst)g(the)e(predictions)h(of)g(the)f (mo)q(dels)i(\(see)d(e.g.)22 b(ref.)15 b([93Borc]\))h(esp)q(ecially)i(along) -47 1637 y(the)13 b(astroph)o(ysical)j(r-pro)q(cess)e(paths.)21 b(And)14 b(y)o(et)e(the)i(longest)h(isotopic)g(c)o(hains)g(kno)o(wn)e(with)i (fair)f(precision)-47 1697 y(\(40)j(k)o(eV\))e(do)h(not)h(exceed)e(33)i(n)o (uclides)g(\(for)f(Pb\))h(or)f(28)h(in)g(the)f(case)h(of)f(Cs.)-47 1793 y(W)l(e)f(m)o(ust,)g(in)h(the)g(\014rst)g(place,)g(men)o(tion)f(the)h (new)f(P)o(enning)i(trap)f(measuremen)o(ts)e([95Hart)q(],)h([95Boll)q(])g(on) -47 1853 y(hea)o(vy)c(Rb,)h(Sr,)g(Cs)g(and)g(Ba)f(isotop)q(es,)j(obtained)f (after)e(the)h(mo)o(v)o(e)e(to)i(the)f(new)g(ISOLDE)h(facilit)o(y)l(.)21 b(They)11 b(led)-47 1913 y(to)17 b(drastically)h(impro)o(v)o(ed)e(accuracies) h(far)g(from)f(stabilit)o(y)l(.)24 b(A)16 b(v)o(ery)g(recen)o(t)f(impro)o(v)o (emen)o(t)g(in)i(the)f(set-up)-47 1973 y([95Raim)q(])h(no)o(w)i(allo)o(ws)i (mass-measuremen)o(ts)d(of)g(some)h(rare-earth)f(n)o(uclides)h(\()1469 1955 y fi(139)p fd(;)p fi(140)p fd(;)p fi(142)p fd(;)p fi(1)o(43)1713 1973 y fm(Sm,)1813 1955 y fi(139)1868 1973 y fm(Eu\),)-47 2033 y(the)14 b(results)h(of)f(whic)o(h)g(are,)h(unfortunately)l(,)f(not)h(y)o(et) e(a)o(v)m(ailable)k(and)d(will)i(not)f(b)q(e)f(included)h(in)g(the)f(coming) -47 2094 y(AME-95)19 b(up)q(date.)29 b(F)l(or)19 b(the)g(ligh)o(ter)g(Rb)g (isotop)q(es,)i(the)d(di\013erences)h(with)h(earlier)f(data)h(on)f(isobaric)i (Sr)-47 2154 y(mass)d(v)m(alues,)h(agree)f(quite)g(w)o(ell)h(with)f(the)g (rep)q(orted)g(v)m(alues)h(for)f(the)g(Rb\()p fe(\014)1408 2136 y fc(\000)1437 2154 y fm(\)Sr)g(deca)o(y)f(energies.)27 b(This)-47 2214 y(mak)o(es)20 b(it)h(ev)o(en)e(more)h(amazing)i(that)f(the)g (new)f(Sr)h(v)m(alues)g(do)g(not)h(agree)e(so)h(w)o(ell)h(with)f(the)f(rep)q (orted)-47 2274 y fe(\014)s fm(-deca)o(y)15 b(energies)h(of)g(these)g(isotop) q(es)i(and)e(their)h(daugh)o(ters.)k(The)16 b(dep)q(endabilit)o(y)i(of)e(the) g(P)o(enning-trap)-47 2334 y(measuremen)o(ts)j(after)i(dismoun)o(ting)i(and)e (reassem)o(bly)g(of)g(the)f(apparatus)i(is)g(assessed)g(b)o(y)e(the)g(p)q (erfect)-47 2395 y(agreemen)o(t)c(obtained)j(for)e(the)g(hea)o(vy)g(Cs)g(and) h(Ba)f(isotop)q(es)i(b)q(efore)f(and)f(after)h(the)f(mo)o(v)o(e.)22 b(In)17 b(our)h(1993)-47 2455 y(mass)k(adjustmen)o(t,)g(the)443 2437 y fi(91)480 2455 y fm(Sr\()p fe(\014)576 2437 y fc(\000)605 2455 y fm(\))g(deca)o(y)e(energy)i(w)o(as)g(already)g(one)g(of)g(the)g(three) f(somewhat)h(sev)o(ere)-47 2515 y(di\016culties)16 b(men)o(tioned)f(in)i (setion)f(3.2)g(of)f([IV)o(].)21 b(V)l(alues)15 b(of)h(2669\(10\))i ([53Am08],)d(2684\(4\))i([73Ha11)q(])e(and)-47 2575 y(2704.5\(3.0\))23 b(k)o(eV)d([80De02)q(])g(w)o(ere)h(rep)q(orted,)h(to)f(whic)o(h)h(one)f (could)h(add)g(the)f(McGill)h(v)m(alue)g(2709\(15\))-47 2635 y([83Ia02)q(];)d(but)g(the)g(new)g(doublets)h(implicate)g(a)g(v)m(alue)f (2730\(10\))j(k)o(eV,)17 b(higher)j(than)f(all)i(of)e(them.)29 b(Re-)-47 2696 y(studying)20 b(the)e(three)g(pap)q(ers)h(men)o(tioned,)g(w)o (e)f(found)i(no)f(reason)g(to)g(distrust)h(the)e(\014rst)h(t)o(w)o(o,)g (measured)-47 2756 y(with)j(magnetic)g(sp)q(ectrometers.)36 b(The)22 b(third)g(w)o(as)g(measured)f(with)h(a)g(semiconductor)g(sp)q (ectrometer;)-47 2816 y(here)c(it)i(is)g(noted)f(that)h(the)f(error)g(ab)q(o) o(v)o(e)g(is)h(the)f(one)g(men)o(tioned)g(in)h(the)f(abstract,)h(but)g(that)f (the)g(text)-47 2876 y(men)o(tions)14 b(errors)h(of)g(5)f(and)h(8)g(k)o(eV.)e (But)h(ev)o(en)f(the)h(latter)h(do)q(es)g(not)g(quite)f(co)o(v)o(er)f(the)h (di\013erence)h(with)g(the)-47 2936 y(mass)k(sp)q(ectrometer)e(result.)28 b(This)20 b(is)f(just)f(one)h(example,)f(alb)q(eit)i(the)e(most)h(w)o (orrisome,)g(of)g(di\016culties)p eop %%Page: 4 4 bop -47 30 a fm(w)o(e)18 b(had)h(with)g(the)f(new)g(v)m(alues.)29 b(Our)18 b(studies,)h(together)g(with)g(that)g(of)f(Hartmann)h([94Hart],)f (led)h(to)f(a)-47 90 y(revision)i(of)g(some)f(error)g(v)m(alues)h(rep)q (orted)f(b)o(y)g(the)g(authors)h(in)g(ref.)e([80De02)q(])h(and)h(of)f(the)g (consistency)-47 150 y(factors)e(\(see)f(b)q(elo)o(w\))h(of)g(some)f(other)g (mass-sp)q(ectrometric)h(data.)23 b(The)16 b(deca)o(y)g(energy)g(of)1675 132 y fi(91)1713 150 y fm(Rb\()p fe(\014)1826 132 y fc(\000)1855 150 y fm(\))g(has)-47 210 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y(n)o(um)o(b)q(er)c(of)i(data)h (that)f(ha)o(v)o(e)e(b)q(ecome)h(a)o(v)m(ailable)j(since.)25 b(Before,)17 b(the)g(rep)q(orted)h(errors)g(w)o(ere)e(m)o(ultiplied)-47 1853 y(with)e(a)f(\\consistency)h(factor")g(of)g(1.5;)g(this)g(v)m(alue)g(no) o(w)f(app)q(ears)h(sligh)o(tly)h(underestimated)f(and)f(w)o(e)g(found)-47 1913 y(it)k(necessary)e(to)i(increase)g(this)g(to)f(2.5.)-47 2009 y(Also)c(the)f(mass)h(measuremen)o(ts)e(of)i(the)f(St-P)o(etersburg)h (group)g(with)h(the)e(PRISM)g(sp)q(ectrometer)f([89Al33)r(],)-47 2069 y(p)q(erformed)16 b(un)o(til)h(no)o(w)g(only)h(for)e(7)h(isotop)q(es)i (of)d(Rb,)g(do)h(not)g(agree)g(w)o(ell)g(with)g(other)g(data,)g(exhibiting)h (a)-47 2129 y(systematic)f(deviation,)i(with)f(an)f(o)o(v)o(erall)h (discrepancy)g(of)f(4.01.)25 b(The)17 b(calibration)j(pro)q(cedure)d(in)h (whic)o(h)-47 2189 y(elemen)o(ts)12 b(\(Zr,)h(Nb,)g(Mo\))g(di\013eren)o(t)g (from)f(the)h(measured)g(Rb)g(w)o(ere)f(used,)h(ma)o(y)g(ha)o(v)o(e)f (resulted)h(in)g(di\013eren)o(t)-47 2249 y(ionization)h(lo)q(cations)g(in)e (the)f(source)g(and)h(ma)o(y)e(b)q(e)i(a)g(reason)g(for)f(suc)o(h)g(an)h (e\013ect.)19 b(No)11 b(other)h(measuremen)o(ts)-47 2310 y(with)20 b(the)f(same)h(sp)q(ectrometer)e(ha)o(v)o(e)h(b)q(een)g(rep)q(orted)h(since)f (then.)31 b(The)19 b(necessary)h(PCF)f(of)h(4)g(is)g(suc)o(h)-47 2370 y(that)c(these)g(data)h(are)g(out)o(w)o(eigh)o(ted)f(b)o(y)g(the)g (ensem)o(ble)f(of)i(all)h(the)e(other)g(ones.)-47 2572 y ff(5.)37 b(New)26 b(reaction)i(and)f(deca)n(y)g(data)-47 2717 y fm(Whereas)15 b(mass-sp)q(ectrometric)h(data)g(almost)g(alw)o(a)o(ys)g(yield)g(exp)q (erimen)o(tal)f(v)m(alues)i(for)e(masses,)g(it)h(is)g(not)-47 2777 y(alw)o(a)o(ys)f(so)h(for)e(energy)h(measuremen)o(ts)e(from)i(deca)o(ys) f(or)h(reactions.)22 b(The)14 b(reason)i(is)f(that)g(it)h(often)e(o)q(ccurs) -47 2837 y(that)i(b)q(oth)i(paren)o(t)e(and)h(daugh)o(ter)f(n)o(uclides)h(in) g(the)f(\014rst)g(case,)g(or)h(target)f(and)h(residual)h(n)o(uclides)f(in)g (the)-47 2897 y(second,)h(ha)o(v)o(e)f(unkno)o(wn)h(masses.)27 b(Therefore)18 b(if)g(a)h(later)f(exp)q(erimen)o(t)f(determines)h(the)f(mass) i(of)f(one)g(of)p eop %%Page: 5 5 bop -47 30 a fm(them,)19 b(the)g(other)h(one)g(is)g(determined)f(at)h(the)g (same)f(time.)31 b(A)19 b(somewhat)i(excellen)o(t)d(example)i(can)g(b)q(e)-47 90 y(found)e(in)g(the)f(determination)h(of)g(the)f(isomeric)h(excitation)h (energy)d(of)1323 72 y fi(181)1378 90 y fm(Os)i(b)o(y)f(the)g(ISOCELE)h (group)-47 150 y([95Rous)q(]:)h(the)14 b(mass)h(of)g(the)f(excited)f(isomer)i (b)q(eeing)g(kno)o(wn)f(from)g(its)h fe(\014)1335 132 y fi(+)1364 150 y fm(-deca)o(y)l(,)f(not)g(only)h(the)f(ground-)-47 210 y(state)j(mass)h(of)250 192 y fi(181)305 210 y fm(Os)f(is)h(no)o(w)g(kno)o (wn,)f(but)g(also)i(the)d(masses)i(of)1192 192 y fi(185)1247 210 y fm(Pt)g(from)f(its)g fe(\013)p fm(-deca)o(y)g(to)h(the)f(latter,)-47 271 y(of)8 252 y fi(185)63 271 y fm(Au)f(from)g(its)h fe(\014)357 252 y fi(+)386 271 y fm(-deca)o(y)f(and)h(of)f(its)h 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fm(126\),)j(where)-47 1003 y(not)g(so)g(man)o(y)f(masses)i(are)e(kno)o(wn,)h(the)f(sev)o(eral)h fe(\013)p fm(-deca)o(y)f(energies)h(measured)g(at)g(RITU)f(help)h(map)g(the) -47 1064 y(region;)g(they)e(are)i(milestone)g(a)o(w)o(aiting)h(connections)f (to)g(the)f(bac)o(kb)q(one)g(of)h(masses.)-47 1159 y(Some)c(v)o(ery)g(hea)o (vy)g(n)o(uclides)h(and)h(more)e(esp)q(ecially)i(new)f(elemen)o(ts)f(\(see)g (section)h(3\))h(ha)o(v)o(e)e(b)q(een)g(iden)o(ti\014ed)-47 1219 y(and)23 b(their)g(half-liv)o(es)h(and)f fe(\013)p fm(-deca)o(y)f (energies)h(determined.)40 b(With)23 b(few)f(exceptions)h(the)f(observ)o(ed)g fe(\013)-47 1280 y fm(lines)e(are)g(not)g(connecting)g(ground-states,)i(but)d (they)g(still)j(giv)o(e)d(useful)h(information)i(in)e(getting)h(go)q(o)q(d) -47 1340 y(estimates)16 b(of)h(the)f fe(Q)346 1347 y fd(\013)387 1340 y fm(energies)g(and)h(masses)g(of)f(the)g(hea)o(viest)g(n)o(uclides.)-47 1484 y fl(5.1.)31 b(Gamma-ra)n(y)22 b(recalibration)-47 1612 y 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y(Notew)o(orth)o(y)g(is)h(the)g(newly)g(rep)q(orted)g(proton)h(energy)e(of) 1068 2564 y fi(112)1123 2582 y fm(Cs)h(whic)o(h)g(is)h(smaller)g(than)f(that) g(in)1838 2564 y fi(113)1893 2582 y fm(Cs,)-47 2642 y(con)o(trary)12 b(to)g(the)g(normal)h(increase)f(with)h(decreasing)g(neutron)f(n)o(um)o(b)q (ers,)g(probably)h(re\015ecting)g(a)f(stronger)-47 2702 y(neutron-proton)k (pairing)g(energy)l(.)21 b(Suc)o(h)14 b(in)o(v)o(ersion)h(is)g(also)i(observ) o(ed)d(for)1358 2684 y fi(108)1413 2702 y fm(I)h(for)g(whic)o(h)f(an)h(upp)q (er)g(limit)-47 2762 y(of)f(500)i(k)o(eV)d(is)i(rep)q(orted)f(for)h(the)f (energy)g(of)h(the)f(emitted)g(protons.)21 b(Moreo)o(v)o(er,)13 b(in)i(the)f(latter)h(case,)f(since)-47 2823 y(this)j(energy)f(m)o(ust)g(b)q (e)g(p)q(ositiv)o(e,)h(w)o(e)f(represen)o(ted)f(this)i(result)g(as)g(a)f (measured)g(v)m(alue.)p eop %%Page: 6 6 bop -47 30 a fl(5.3.)31 b(Other)23 b(deca)n(ys)g(and)g(reactions)-47 158 y fm(Since)f(the)g(AME-93)g(new)g fe(\013)p 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(di\013eren)o(tial)i(reaction)e(energies)g(p)q(erformed)g(at)g(Heidelb)q(erg) g(on)-47 596 y fi(40)-10 614 y fm(Ar,)i(and)h(b)o(y)f(the)g(T)q(\177)-26 b(ubingen-Indiana)23 b(group)d(on)g(Hg)f(isotop)q(es.)32 b(Also,)20 b(thermal)g(neutron)f(capture)g fe(\015)s fm(-)-47 675 y(deca)o(ys,)d(that)h (pro)o(vide)h(some)e(of)i(the)f(most)g(precise)g(data,)g(ha)o(v)o(e)f(b)q (een)h(rep)q(orted)g(b)o(y)g(groups)h(at)g(ILL)f(and)-47 735 y(Latvia,)g(for)g(Ni)f(and)h(Ba)f(isotop)q(es.)-47 879 y fl(5.4.)31 b(Final)24 b(lev)n(els)f(in)g fa(\013)p fl(-deca)n(y)-47 1007 y fm(In)e fe(\013)p fm(-deca)o(y)l(,)i(the)f(energy)f(of)h(emitted)g fe(\013)p fm(-particles)h(is)g(usually)h(measured)d(with)i(go)q(o)q(d)h (accuracy)l(.)38 b(F)l(or)-47 1067 y(n)o(uclides)21 b(with)g(an)f(ev)o(en)f (n)o(um)o(b)q(er)h(of)g(protons)i(and)e(of)h(neutrons,)g(the)f(strongest)h (branc)o(h)g(alw)o(a)o(ys)g(go)q(es)-47 1127 y(to)g(the)f(ground-state)j(of)e (the)f(daugh)o(ter.)35 b(Unfortunately)l(,)22 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y(di\013eren)o(t)h(from)g(that)h(used)g(for)f(systematics)h(\(#\).)30 b(This)21 b(p)q(olicy)f(will)h(b)q(e)f(generalized)g(in)g(the)f(AME-95)-47 2005 y(up)q(date.)-47 2101 y(Unfortunately)l(,)h(the)f(systematics)h(of)g (Nilsson)h(assignmen)o(ts)f(to)g(n)o(uclides)g(with)h(o)q(dd)f(n)o(um)o(b)q (ers)f(b)q(oth)h(of)-47 2161 y(protons)k(and)f(neutrons)g(is)h(more)e (complicated.)42 b(W)l(e)22 b(did)i(not)f(try)g(to)g(mak)o(e)f(a)h(similar)h (analysis)h(for)-47 2221 y(them.)d(A)16 b(\014rst)h(review)f(of)h(the)f (deformed)h(region)g fe(A)p fm(=155{185)i(seems)d(to)h(indicate)h(that)f (extrap)q(olations)-47 2282 y(of)f(excitation)i(energies)e(of)h(Nilsson)h (lev)o(els)e(are)g(less)h(dep)q(endable)g(here.)-47 2426 y fl(5.5.)31 b(The)231 2404 y fj(10)274 2426 y fl(Li)24 b(ground-state)g(mass) -47 2554 y fm(The)15 b(imp)q(ortan)o(t)h(question)g(of)f(whic)o(h)h(state)f (is)h(the)f(ground-state)i(often)e(o)q(ccurs)h(in)f(the)g(mass)h(ev)m (aluation.)-47 2614 y(An)23 b(example)h(is)h(giv)o(en)f(b)o(y)506 2596 y fi(10)543 2614 y fm(Li,)j(whic)o(h)d(is)g(un)o(b)q(ound)h(to)f (particle)h(emission)g(and)g(whose)f(states)h(are)-47 2674 y(observ)o(ed)18 b(as)i(resonances.)29 b(Masses)20 b(ha)o(v)o(e)e(b)q(een)h (measured)f(in)i(recen)o(t)d(exp)q(erimen)o(ts)i(at)g(MSU)f([94Y)l(o01)q(]) -47 2734 y(and)h(at)g(HMI)e([95Bohl)q(].)28 b(The)18 b(apparen)o(t)h (discrepancy)g(among)g(their)g(results,)g(and)g(also)i(with)e(previous)-47 2795 y(studies,)24 b(are)e(due)g(to)h(the)f(di\013eren)o(t)g(selectivities)i (of)e(the)g(reactions)i(used.)39 b(The)22 b(mass)h(measured)f(b)o(y)-47 2855 y([95Bohl)q(])17 b(at)h(240\(60\))h(k)o(eV)d(ab)q(o)o(v)o(e)h(the)h(one) f(neutron)h(threshold)h(unam)o(biguously)g(corresp)q(onds)g(to)f(a)g(1)1931 2837 y fi(+)-47 2915 y fm(state)f(with)g(the)g(con\014guration)i(of)e(a)g(1p) 713 2897 y fi(1)p fd(=)p fi(2)785 2915 y fm(neutron)g(resonance)g(coupled)g (to)h(the)e(3/2)1586 2897 y fc(\000)1617 2915 y fm(core)g(of)1776 2897 y 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(should)f(b)q(e)g(later)f(pro)o(v)o(ed)-47 883 y(not)g(to)h(b)q(e)f(a)h (resonance,)f(the)g(ground-state)i(mass)f(w)o(ould)g(b)q(e)f(some)h(200)g(k)o (eV)e(higher.)-47 1028 y fl(5.6.)90 1006 y fj(99)134 1028 y fl(Rh)22 b(isomers)-47 1155 y fm(A)c(new)h(publication)i([94Kuma])d (con\014rms)h(an)g(earlier)h(one)f(of)g([69Ph01)q(],)f(that)i(the)e(4.7)h(h)g (9/2)1773 1137 y fi(+)1822 1155 y fm(isomer)-47 1216 y(in)11 1197 y fi(99)48 1216 y fm(Rh)f(is)g(64.3\(.4\))h(k)o(eV)d(ab)q(o)o(v)o(e)h (the)h(16.1)g(d)g(1/2)906 1197 y fc(\000)954 1216 y fm(one.)25 b(F)l(or)18 b(this)h(reason)f(w)o(e)f(restudied)h(the)f(a)o(v)m(ailable)-47 1276 y(publications)g(on)e(the)g(deca)o(y)e(of)i(the)g(latter)g(one,)g(for)g (whic)o(h)g(w)o(e)f(\014rst)h(accepted)f(the)g([74An23)q(])g(conclusion)-47 1336 y(that)21 b(its)g(deca)o(y)f(energy)h(is)g(larger)h(than)f(that)g(of)g (the)g(former;)h(the)e(data)i(of)f([59T)l(o)o(wn)q(],)g(giv)o(en)f(only)i(in) -47 1396 y(an)d(abstract,)i(w)o(e)d(trusted)h(less.)31 b(Considering)22 b(no)o(w)d(their)g(rather)h(extensiv)o(e)e fe(\015)s fm(-)p fe(\014)k fm(coincidence)d(data)h(in)-47 1456 y(com)o(bination)12 b(with)g(the)e(mo)q(dern)i(deca)o(y)e(sc)o(heme)f([NDS],)i(w)o(e)f(noticed)h (that)h(the)e(deca)o(y)g(energies)i(calculated)-47 1516 y(from)i(the)h(four)g ([59T)l(o)o(wn)q(])f fe(\014)s fm(-branc)o(hes)h(agreed)g(excellen)o(tly)f (and)i(that)f(the)f(lo)o(w)o(er)h(branc)o(hes)g(found)g(in)h(the)-47 1577 y(singles)23 b fe(\014)s fm(-sp)q(ectrum)e(b)o(y)f([74An23)q(])h(m)o (ust)g(b)q(e)g(considered)h(mixtures)g(and)g(therefore)e(should)j(b)q(e)f (giv)o(en)-47 1637 y(little)15 b(w)o(eigh)o(t.)20 b(A)13 b(happ)o(y)h (consequence)f(of)g(the)h(resulting)h(c)o(hanges)f(is)g(that)g(some)g (earlier)g(bad)g(agreemen)o(ts)-47 1697 y(with)j(other)f(data)h(almost)h (disapp)q(ear.)-47 1793 y(It)h(is)i(in)o(teresting)f(to)g(note)g(that)g(the)g fe(J)709 1775 y fd(\031)752 1793 y fm(systematics)g(\(see)f(section)h(6\))g (of)g(ground-states)i(and)e(excited)-47 1853 y(isomers)15 b(for)f(o)q(dd-)p fe(Z)t fm(,)h(ev)o(en-)p fe(N)k fm(n)o(uclides)c(in)f(this)h(region)h(do)e (not)h(sho)o(w)g(a)f(preference)f(for)h(either)g(of)h(the)f(t)o(w)o(o)-47 1913 y(alternativ)o(es)j(for)f(the)374 1895 y fi(99)412 1913 y fm(Rh)g(isomers.)-47 2115 y ff(6.)37 b(T)-7 b(reatmen)m(t)25 b(of)j(excitation)g(energies)g(of)g(isomers)-47 2260 y fm(The)16 b(excitation)h(energy)f(of)h(an)f(isomer)h(is)g(deriv)o(ed)f(either)g(from)g (in)o(ternal)i(energy)d(relations,)j(most)f(often)-47 2320 y(a)e fe(\015)s fm(-deca)o(y)f(or)h(a)g(com)o(bination)h(of)f fe(\015)j fm(energies,)d(or)g(from)f(external)h(energy)f(relations,)j(lik)o (e)e(particle)g(deca)o(ys)-47 2380 y(or)k(reaction)h(energies.)29 b(Whereas)19 b(the)g(n)o(uclear)g(structure)f(ev)m(aluators)j(are)e(the)f (most)h(quali\014ed)h(to)g(giv)o(e)-47 2440 y(v)m(alues)g(for)g(the)f (excitation)h(energies)g(of)g(the)f(\014rst)g(category)l(,)h(the)f(AME)g(can) h(b)q(est)f(giv)o(e)h(v)m(alues)g(for)g(the)-47 2501 y(second.)28 b(Up)19 b(to)g(no)o(w)g(w)o(e)f(w)o(ere)g(in)o(terested)g(only)i(in)f(those)g (isomers)h(whic)o(h)f(w)o(ere)e(essen)o(tial)j(in)g(deriving)-47 2561 y(the)c(ground-state)h(masses:)22 b(those)16 b(w)o(ere)f(the)h(cases)h (where)e(exp)q(erimen)o(tal)h(data)h(allo)o(w)o(ed)h(determination)-47 2621 y(of)e(the)g(masses)h(of)f(b)q(oth)h(states.)22 b(If)16 b(the)g(excitation)h(energy)f(of)g(the)g(upp)q(er)g(lev)o(el)g(w)o(as)h(kno)o (wn)g(from)f fe(\015)s fm(-ra)o(y)-47 2681 y(measuremen)o(ts,)c(its)h(com)o (bination)h(with)f(the)g(mass)g(of)g(the)f(upp)q(er)h(lev)o(el)f(lead)h(to)g (a)g(more)g(accurate)f(v)m(alue)h(of)-47 2741 y(the)i(mass)i(of)f(the)f (ground)i(state.)k(If)15 b(not,)h(the)g(data)g(men)o(tioned)g(presen)o(ted)f (the)g(b)q(est)h(a)o(v)m(ailable)j(estimate)-47 2802 y(of)d(the)g(excitation) i(energy)d(of)i(the)f(upp)q(er)g(isomer.)-47 2897 y(Our)d(presen)o(t)f(p)q (olicy)l(,)i(discussed)g(with)g(ENSDF)f(ev)m(aluators,)h(is)g(to)f(include)h (in)f(our)h(ev)m(aluation)h(all)f(isomers)p eop %%Page: 8 8 bop -47 30 a fm(for)21 b(whic)o(h)h(the)e(excitation)j(energy)d(is)i(not)g (deriv)o(ed)e(from)h fe(\015)s fm(-ra)o(y)h(measuremen)o(ts,)e(and)i(also)h (those)e(for)-47 90 y(whic)o(h)c(the)g(precision)i(in)e fe(\015)s fm(-ra)o(y)h(measuremen)o(ts)e(is)i(not)f(decidedly)h(b)q(etter)f(than)g (that)h(of)f(particle)h(deca)o(y)-47 150 y(or)e(reaction)h(energies)g (leading)h(to)e(them.)-47 246 y(Also,)k(to)f(b)q(e)h(consisten)o(t,)g(those)f (v)o(ery)f(precise)h(excitation)i(energies)e(deriv)o(ed)g(from)g fe(\015)s fm(-energy)g(measure-)-47 306 y(men)o(ts)14 b(should)j(b)q(e)f (treated)f(in)h(the)f(AME)g(as)h(an)o(y)g(other)f(lev)o(el)h(en)o(tering)f(a) h(reaction)g(or)g(a)g(deca)o(y)e(relation,)-47 366 y(i.e.)20 b(their)c(v)m(alue)f(should)i(b)q(e)e(added)g(to)h(or)f(substracted)h(from)f (the)f(measured)h(energy)g(to)g(yield)h(a)f(ground-)-47 426 y(state)20 b(to)g(ground-state)i(energy)l(.)32 b(Our)20 b(general)h(p)q (olicy)h(in)e(a)o(v)o(eraging)h(energy)f(lines)h(of)f(di\013eren)o(t)h(lev)o (els)-47 487 y(\(in)16 b(the)g(same)g(deca)o(y)f(or)h(reaction)h(and)f(in)h (a)f(giv)o(en)g(exp)q(erimen)o(t\))f(is)i(to)f(assign)i(to)e(the)g(a)o(v)o (erage)f(the)h(error)-47 547 y(of)21 b(the)g(most)h(precise)f(item,)g (instead)i(of)e(the)g(error)g(on)h(the)f(a)o(v)o(erage,)g(pro)o(vided)h (these)f(errors)g(are)g(not)-47 607 y(dominated)15 b(b)o(y)f(statistics.)22 b(This)16 b(a)o(v)o(oids)f(giving)h(an)f(o)o(v)o(er-optimistic)g(result)g (for)f(that)h(deca)o(y)f(or)g(reaction.)-47 667 y(The)f(new)h(treatmen)o(t)e (of)i(the)g(v)o(ery)e(precisely)i(kno)o(wn)f(isomeric)i(excitation)f (energies)g(p)q(ermits)g(us)g(to)g(apply)-47 727 y(the)i(ab)q(o)o(v)o(e)g(p)q (olicy)i(to)e(them)g(also)i(and)e(th)o(us)h(to)f(repair)h(a)g(sligh)o(t)h (defect)d(in)i(the)f(previous)h(ev)m(aluations.)-47 872 y fl(6.1.)31 b(Uncertain)23 b(assignmen)n(ts)f(for)i(isomers)-47 1000 y fm(In)18 b(some)g(cases)g(the)g(v)m(alue)h(determined)e(b)o(y)h(the)g(AME)f (for)i(the)e(isomeric)i(excitation)g(energy)f(allo)o(ws)i(no)-47 1060 y(decision)i(as)g(to)g(whic)o(h)f(of)h(the)f(t)o(w)o(o)g(is)h(the)e (ground-state.)38 b(This)22 b(is)g(particularly)h(the)e(case)h(when)f(the)-47 1120 y(uncertain)o(t)o(y)16 b(on)g(the)g(excitation)i(energy)d(is)i(large)h (compared)e(to)g(that)h(energy)l(,)e(e.g.:)35 1180 y fe(E)74 1162 y fd(m)108 1180 y fm(\()127 1162 y fi(82)164 1180 y fm(As\))f(=)g(140)8 b fb(\006)g fm(200)16 b(k)o(eV;)95 b fe(E)752 1162 y fd(m)785 1180 y fm(\()804 1162 y fi(134)859 1180 y fm(Sb\))15 b(=)f(50)8 b fb(\006)g fm(150)15 b(k)o(eV;)95 b fe(E)1421 1162 y fd(m)1455 1180 y fm(\()1474 1162 y fi(154)1529 1180 y fm(Pm\))14 b(=)g(50)8 b fb(\006)g fm(130)15 b(k)o(eV)-47 1240 y(In)f(the)h(ab)q(o)o(v)o(e)f (examples)h(all)h(3)f(n)o(uclides)h(are)f(o)q(dd-o)q(dd)i(where)d(in)h (general)h(the)e(trends)h(in)g fe(J)1679 1222 y fd(\031)1717 1240 y fm(systematics)-47 1300 y(are)i(of)g(no)g(help.)23 b(Neither)16 b(could)i(an)o(y)f(preference)e(for)i(ground-state)h(or)f(excited)g(state)g (b)q(e)f(deriv)o(ed)h(from)-47 1361 y(n)o(uclear)f(structure)g(data.)22 b(The)16 b(assignmen)o(t)i(w)o(e)d(adopted)i(is)g(suc)o(h)f(that)h(the)f(v)m (alue)h(for)g fe(E)1660 1343 y fd(m)1709 1361 y fm(is)g(p)q(ositiv)o(e.)-47 1456 y(Otherwise,)f(if)h(an)g(ordering)h(is)f(indicated)g(b)o(y)f(n)o(uclear) h(structure)f(\(e.g.)22 b(if)16 b(one)h(of)g(the)f(isomers)h(is)g(kno)o(wn) -47 1516 y(to)f(deca)o(y)f(in)o(to)i(the)e(other)h(one,)g(or)g(if)h(the)e (Gallagher-Mosk)o(o)o(wski)k(rule)d(for)g(relativ)o(e)g(p)q(ositions)j(of)d (com)o(bi-)-47 1577 y(nations)k(p)q(oin)o(t)g(strongly)g(to)f(one)f(of)h(the) g(t)o(w)o(o)f(as)h(b)q(eing)h(the)f(ground-state\),)h(or)f(if)g(a)g(prefered) e(ordering)-47 1637 y(could)h(b)q(e)f(deriv)o(ed)f(from)h(the)g(trends)g(of)g (systematics)g(in)h fe(J)1079 1619 y fd(\031)1102 1637 y fm(,)e(w)o(e)h(tak)o (e)f(suc)o(h)h(constrain)o(ts)h(in)o(to)g(consider-)-47 1697 y(ation.)31 b(In)19 b(the)g(\014rst)g(case)h(the)f(distribution)i(of)f (probabilit)o(y)h(is)f(truncated)f(and)h(only)g(its)g(p)q(ositiv)o(e)g(part) -47 1757 y(is)g(accepted.)31 b(In)19 b(the)h(second)f(case,)h(the)g(ordering) h(suggested)f(b)o(y)f(systematics)h(is)h(accepted)e(ev)o(en)f(if)i(it)-47 1817 y(ma)o(y)g(yield)i(a)f(\(sligh)o(tly\))i(negativ)o(e)e(v)m(alue)h(for)g (the)f(excitation)h(energy)l(,)f(e.g.)35 b({60)p fb(\006)p fm(110)24 b(k)o(eV)19 b(for)1843 1799 y fi(108)1898 1817 y fm(Rh)-47 1878 y(or)f({20)p fb(\006)p fm(50)h(k)o(eV)e(for)369 1860 y fi(124)424 1878 y fm(In.)25 b(Suc)o(h)18 b(systematics)g(are)g(still)h (more)f(useful)g(for)g(o)q(dd-)p fe(A)h fm(n)o(uclides,)f(for)g(whic)o(h)-47 1938 y(isomeric)j(excitation)h(energies)f(of)f(isotop)q(es)j(\(if)e fe(N)26 b fm(is)21 b(ev)o(en\))f(or,)h(similarly)l(,)j(isotones)e(follo)o(w)g (usually)g(a)-47 1998 y(systematic)e(course.)31 b(This)21 b(allo)o(ws)h(to)e (deriv)o(e)f(estimates)h(b)q(oth)g(for)g(the)g(relativ)o(e)f(p)q(osition)k (and)d(for)g(the)-47 2058 y(excitation)d(energies)g(where)e(they)h(are)g(not) h(kno)o(wn.)-47 2203 y fl(6.2.)31 b(Some)22 b(particular)i(isomers)-47 2330 y fg(Isomers)c(in)230 2312 y fi(137)285 2330 y fg(Pm:)25 b fm(The)18 b(p)q(ossible)j(existence)c(of)i(isomers)g(ma)o(y)e(cause)i(an)f (uncertain)o(t)o(y)g(in)h(the)f(mass)-47 2391 y(assigned)h(to)g(the)e (ground-state.)28 b(An)18 b(example)f(migh)o(t)h(b)q(e)g(found)h(in)1284 2373 y fi(137)1339 2391 y fm(Pm,)e(for)h(whic)o(h)h(Gromo)o(v)f(et)f(al.)-47 2451 y([95Grom])g(rep)q(ort)h(a)g fe(\014)390 2433 y fi(+)419 2451 y fm(-deca)o(y)e(of)i(its)g(2.4)g(m)f(high-spin)i(isomer.)25 b(In)17 b(the)g(isotop)q(es)j(of)d(this)h(n)o(uclide,)g(the)-47 2511 y(11/2)49 2493 y fc(\000)97 2511 y fm(lev)o(els)f(are)f(the)h(upp)q(er)g (isomers.)24 b(Y)l(et,)15 b(extrap)q(olation)20 b(of)d(their)g(lev)o(el)g (energies,)g(and)g(also)h(consid-)-47 2571 y(eration)i(of)f(their)g(half-liv) o(es,)i(suggest)f(that)g(it)f(could)h(also)g(b)q(e)g(the)e(ground-state)j(in) 1591 2553 y fi(137)1646 2571 y fm(Pm.)29 b(Moreo)o(v)o(er)-47 2631 y(no)18 b(isomeric)g(activit)o(y)g(is)h(kno)o(wn)e(for)h(this)h(n)o (uclide.)26 b(W)l(e)17 b(treat)h(nev)o(ertheless)f(its)h(data)h(as)f(a)g (deca)o(y)f(from)-47 2692 y(an)e(isomeric)h(state)f(lo)q(cated)g(at)h(an)f (estimated)g(energy)f(of)h(0#)p fb(\006)p fm(100)h(k)o(eV)d(to)j(tak)o(e)e (the)g(ab)q(o)o(v)o(e)h(uncertain)o(t)o(y)-47 2752 y(in)o(to)i(accoun)o(t.) -47 2847 y fg(Isomers)h(in)227 2829 y fi(167)282 2847 y fg(Ir)h(and)h(in)g (its)g fe(\013)p fg(-daugh)n(ters:)j fm(Another)17 b(case)g(are)g(the)f fe(\013)p fm(-deca)o(y)h(sequences)f(starting)-47 2908 y(with)h(the)f(t)o(w)o (o)g(isomers)h(of)469 2889 y fi(167)524 2908 y fm(Ir)f(rep)q(orted)h(at)f (this)h(conference)f([95Da)o(vi].)21 b(The)16 b(proton)i(deca)o(ys)d (strongly)p eop %%Page: 9 9 bop -47 30 a fm(suggest)24 b(that)g(the)f(activities)h(in)g(the)f fe(\013)p fm(-series)h(kno)o(wn)g(b)q(efore)f(b)q(elong)i(in)f(realit)o(y)g (to)f(upp)q(er)h(isomers)-47 90 y(\(except,)18 b(curiously)l(,)i(for)f(the)g (\014nal)h(mem)o(b)q(er)827 72 y fi(151)882 90 y fm(Tm\).)29 b(This)20 b(leads)g(to)f(a)g(revision)h(of)f(the)g(ground-state)-47 150 y(masses)d(in)h(this)g(series)g(but)f(also)i(suggests)g(that)e(more)g(of) h(suc)o(h)f(cases)g(m)o(ust)g(b)q(e)h(presen)o(t.)-47 246 y fg(Isomers)h(in)225 228 y fi(190)280 246 y fg(Re:)j fm(The)c(isomeric)g (excitation)g(energy)f(v)m(alue)i(deriv)o(ed)d(from)i(di\013erences)f(in)h fe(\014)1796 228 y fc(\000)1825 246 y fm(-deca)o(y)-47 306 y(energy)12 b(is)i(210)p fb(\006)p fm(290)g(k)o(eV.)d(F)l(rom)i(n)o(uclear)g (structure)f(data)i([NDS)o(])f(it)g(is)g(also)i(kno)o(wn)e(that)g(the)f(6) 1744 288 y fc(\000)1787 306 y fm(isomeric)-47 366 y(state)f(should)i(lie)f (ab)q(o)o(v)o(e)f(the)h(3)514 348 y fc(\000)555 366 y fm(lev)o(el)f(at)h (119.12)g(k)o(eV,)e(resulting)j(in)f(a)g(lo)o(w)o(er)f(limit.)21 b(Theoretical)12 b(estimates)-47 426 y(rep)q(orted)19 b(in)h([NDS)o(])f(giv)o (e)g(isomeric)h(excitation)g(energy)e(v)m(alues)i(of)g(173)g(and)g(220)g(k)o (eV.)d(Th)o(us,)j(it)f(seems)-47 487 y(reasonable)e(to)g(assume)f(an)h(upp)q (er)f(limit)h(of)g(300)g(k)o(eV.)d(F)l(rom)i(a)g(uniform)h(distribution)i(of) d(probabilit)o(y)i(in)-47 547 y(the)c(so)h(de\014ned)g(allo)o(w)o(ed)h(range) f(119{300)i(k)o(eV,)c(w)o(e)h(deriv)o(e)g(an)h(energy)g(210)p fb(\006)p fm(50)h(k)o(eV,)d(in)i(agreemen)o(t)f(with)-47 607 y(all)j(of)g(the)f(ab)q(o)o(v)o(e)g(information.)-47 703 y fg(Isomers)21 b(in)231 684 y fi(248)286 703 y fg(Bk:)k fm(In)19 b(the)f(AME-93)i(w)o(e)e(considered)h(the)f(1)1171 684 y fc(\000)1220 703 y fm(isomer)h(to)g(b)q(e)g(the)g(ground-state)h(and)-47 763 y(deriv)o(ed)e(an)h(excitation)h(energy)e(of)h(20)p fb(\006)p fm(50)h(k)o(eV)d(for)i(the)g(6)1085 745 y fi(+)1133 763 y fm(isomer,)h(from)e (a)h(com)o(bination)i(of)e fe(\014)1835 745 y fc(\000)1882 763 y fm(and)-47 823 y fe(\013)f fm(energies.)26 b(This)19 b(result)f(do)q(es)h(not)f(agree)g(with)h(the)e(n)o(uclear)h(structure)g(ev)m (aluation)i([NDS)o(])d(where)h(the)-47 883 y(6)-23 865 y fi(+)22 883 y fm(state)d(is)g(considered)h(as)f(the)g(ground-state:)22 b(its)16 b(long)g(half-life)h(\(more)d(than)i(9)f(y)o(ears\))g(places)g(it)h (b)q(elo)o(w)-47 943 y(the)g(8)61 925 y fc(\000)107 943 y fm(state,)g(whic)o (h)h(in)g(turn)f(should)i(b)q(e)f(b)q(elo)o(w)g(the)f(1)1013 925 y fc(\000)1059 943 y fm(state)h(from)f(the)g(Gallagher-Mosk)o(o)o(wski)k (rules.)-47 1003 y(The)e(excitation)i(energy)e(men)o(tioned)h(w)o(as)g(deriv) o(ed)f(from)h(the)f(assumption)i(that)f(the)g fe(\013)p fm(-deca)o(y)f(of) 1853 985 y fi(252)1908 1003 y fm(Es)-47 1064 y(\(spin-parit)o(y)e(probably)g (5)444 1046 y fc(\000)474 1064 y fm(\))e(feeds)h(the)f(high)i(spin)g(isomer)f (in)1126 1046 y fi(248)1181 1064 y fm(Bk.)20 b(It)14 b(is)i(not)f(to)g(b)q(e) g(exp)q(ected,)e(though,)-47 1124 y(that)j(the)g(ground-states)i(in)502 1106 y fi(252)557 1124 y fm(Es)f(and)720 1106 y fi(248)775 1124 y fm(Bk)f(ha)o(v)o(e)f(the)h(same)g(Nilsson)h(mo)q(del)g (con\014gurations)h(and)f(the)-47 1184 y(alpha-deca)o(y)23 b(to)g(the)383 1166 y fi(248)438 1184 y fm(Bk)f(rather)g(probably)i(will)g (feed)e(a)h(5)1161 1166 y fc(\000)1213 1184 y fm(lev)o(el)f(ab)q(o)o(v)o(e)g (the)h(ground)g(state.)40 b(W)l(e)-47 1244 y(therefore)21 b(no)o(w)i(assume)f (that)g(this)h fe(\013)p fm(-deca)o(y)f(is)h(follo)o(w)o(ed)g(b)o(y)f(a)g (transition,)k(for)c(whic)o(h)g(w)o(e)g(assume)g(a)-47 1304 y(reasonable)17 b(energy)l(.)-47 1506 y ff(7.)38 b(Regularit)n(y)29 b(of)g(the)f(m)o(ass)o(-surface)d(and)j(use)f(of)i(system)n(atic)-47 1598 y(trends)-47 1743 y fm(It)13 b(is)h(w)o(ell)g(kno)o(wn)g(that)f(the)g (mass-surface)i(exhibits)f(a)g(v)o(ery)e(regular)i(b)q(eha)o(vior)h(with)f (some)f(sup)q(erimp)q(osed)-47 1803 y(\\irregularities".)35 b(Series)21 b(of)f(irregularities)i(that)f(could)g(b)q(e)f(observ)o(ed)f(for) h(sev)o(eral)g fe(Z)k fm(at)c(the)g(same)g fe(N)5 b fm(-)-47 1863 y(n)o(um)o(b)q(er)12 b(or)h(for)g(sev)o(eral)g fe(N)18 b fm(at)13 b(the)f(same)h fe(Z)t fm(-n)o(um)o(b)q(er)f(are)h(considered)g(as) g(\\structures")h(\(shell)g(or)f(subshell-)-47 1923 y(closures,)19 b(shap)q(e)h(transitions\),)h(whereas)e(single)h(irregularities)h(could)f(b)q (e)f(called)g(\\acciden)o(ts".)30 b(Among)-47 1983 y(the)11 b(latter)i(are)e(cases)h(where)g(the)f(result)i(is)f(deriv)o(ed)g(from)f (one,)i(t)o(w)o(o)e(or)h(\(in)h(one)f(case\))f(three)h(measuremen)o(ts)-47 2043 y(of)k(the)g(same)g(ph)o(ysical)i(quan)o(tit)o(y)l(,)d(all)j(div)o (erging)f(from)f(the)g(men)o(tioned)g(regularit)o(y)h(and)g(whic)o(h)g(w)o (ere)e(not)-47 2104 y(con\014rmed)f(b)o(y)g(a)h(di\013eren)o(t)g(metho)q(d.) 21 b(Only)15 b(these)f(cases)h(are)g(concerned)f(here.)20 b(They)15 b(can)f(b)q(e)h(considered)-47 2164 y(as)f(incen)o(tiv)o(es)g(to)g(remeasure) f(the)h(masses)g(of)g(the)g(in)o(v)o(olv)o(ed)f(n)o(uclei)i(\(and)f(of)g (their)g(neigh)o(b)q(ors\),)i(preferably)-47 2224 y(b)o(y)h(di\013eren)o(t)i (metho)q(ds,)f(in)h(order)f(to)g(remo)o(v)o(e)f(an)o(y)h(doubt)h(and)f(p)q (ossibly)j(p)q(oin)o(t)e(out)f(true)g(irregularities)-47 2284 y(due)e(to)h(real)f(ph)o(ysical)i(e\013ects.)-47 2380 y(F)l(ollo)o(wing)j (the)d(new)h(p)q(olicy)h(de\014ned)f(in)g(the)f(AME-93)i(\(ref.)d([I)o(],)i (section)g(4\),)g(w)o(e)g(con)o(tin)o(ue)f(and)h(extend)-47 2440 y(our)h(w)o(ork)f(in)h(\015agging)i(clearly)e(these)f(\\acciden)o(ts".) 31 b(In)19 b(AME-93,)i(w)o(e)e(limited)h(this)g(action)h(mainly)f(to)-47 2500 y(exp)q(erimen)o(tal)d(data)h(for)f(suc)o(h)g(cases,)g(published)h(in)g (regular)g(refereed)e(journals.)25 b(In)16 b(the)h(coming)h(AME-)-47 2560 y(95)j(up)q(date)g(man)o(y)f(data)h(that)g(app)q(eared)h(in)f(other)f(t) o(yp)q(es)g(of)h(publication)i(will)g(b)q(e)d(similarly)j(included)-47 2621 y(with)17 b(the)f(same)h(sp)q(ecial)h(\015ag)f(\(data-\015ag)i(`D'\).)c (This)i(\015ag)h(allo)o(ws)g(to)f(rep)q(eat)g(an)g(adjustmen)o(t)f(with)h (them)-47 2681 y(included,)f(in)h(order)g(to)f(deriv)o(e)g(the)g(series)h(of) f(tables)h(of)g(\\purely)g(exp)q(erimen)o(tal)f(data".)-47 2776 y(It)h(w)o(orth)i(men)o(tioning)g(that)f(t)o(w)o(o)g(cases)g(in)h(the)e (AME-93)i(for)f(whic)o(h)g(w)o(e)g(could)h(pro)o(vide)f(a)g(b)q(etter)g (\\rec-)-47 2837 y(ommended)13 b(v)m(alue",)i(are)f(withdra)o(wn,)i(and)e(a)h (third)f(is)h(under)f(reconsideration.)22 b(In)14 b(the)1624 2819 y fi(90)1661 2837 y fm(Tc\()p fe(\014)1768 2819 y fc(\000)1797 2837 y fm(\)-deca)o(y)l(,)-47 2897 y(com)o(bination)i(of)f(the)f(w)o(ork)h (of)g(Ia\014gliola)j(et)c(al.)22 b([74Ia01)q(])14 b(with)i(later)f(data)g (suggested)h(that)f(the)f(rep)q(orted)p eop %%Page: 10 10 bop -47 30 a fe(\014)s fm(-endp)q(oin)o(t)15 b(b)q(elongs)i(to)f(a)f (mixture)g(of)g(transitions)j(to)d(the)g(ground-state)i(\(22\045\))e(and)h (to)f(the)g(948.1)h(k)o(eV)-47 90 y(excited)g(lev)o(el.)23 b(This)18 b(remo)o(v)o(ed)e(the)g(earlier)i(acciden)o(t.)23 b(The)1106 72 y fi(108)1161 90 y fm(Mo\()p fe(\014)1280 72 y fc(\000)1309 90 y fm(\)-deca)o(y)16 b(has)i(b)q(een)f(con\014rmed)f(b)o(y) -47 150 y(a)i(group)g(in)g(Jyv\177)-24 b(askyl\177)g(a.)25 b(It)17 b(urged)h(us)g(to)f(re-examine)h(the)f(surface)g(of)h(masses)g(in)g (this)g(region)g(to)g(try)f(to)-47 210 y(accomo)q(date)e(this)h(constrain)o (t.)22 b(No)15 b(conclusions)i(ha)o(v)o(e)e(y)o(et)f(b)q(een)h(dra)o(wn.)21 b(Consideration)d(of)d(the)g(rep)q(orts)-47 271 y(on)20 b(the)g fe(\014)143 252 y fc(\000)172 271 y fm(-deca)o(y)g(of)387 252 y fi(204)442 271 y fm(Au)g(sho)o(w)o(ed)g(that)h(the)f(accepted)f(deca)o(y)g (energy)h(b)q(elonged)h(to)g(a)f(4)h(s)f(activit)o(y)-47 331 y(whereas)14 b(later)h(only)g(a)f(ten)g(times)g(longer)h(half-life)h(w)o(as)f (found)f(connected)g(with)h(this)g(n)o(uclide.)21 b(This)15 b(data)-47 391 y(is)i(no)o(w)f(\015agged)i(`F')d(and)i(replaced)f(b)o(y)g(a)h (systematic)f(estimate.)-47 605 y(W)l(e)g(wish)i(to)f(thank)g(our)g(man)o(y)f (colleagues)j(who)e(sen)o(t)f(us)h(their)g(results)h(b)q(efore)e (publication,)j(and)e(those)-47 665 y(with)f(whom)g(w)o(e)f(ha)o(v)o(e)g(had) h(useful)g(and)g(in)o(teresting)g(discussions,)i(more)d(particularly)i(P)l (.G.)e(Hansen)h(and)-47 725 y(G.)g(Bohlen)g(in)h(discussing)i(the)555 707 y fi(10)592 725 y fm(Li)e(puzzle.)-47 927 y ff(References)-47 1057 y fm([I])164 b(G.)16 b(Audi)g(and)h(A.H.)e(W)l(apstra,)i fn(Nucl.)h(Phys.)e fg(A565)h fm(\(1993\))g(1.)-47 1122 y([I)q(I])145 b(G.)16 b(Audi)g(and)h(A.H.)e(W)l(apstra,)i fn(Nucl.)h(Phys.)e fg(A565)h fm(\(1993\))g(66.)-47 1188 y([I)q(I)q(I])126 b(C.)16 b(Borcea,)f(G.)h(Audi,)g(A.H.)f(W)l(apstra)i(and)g(P)l(.)f(F)l(a)o(v)m(aron,) g fn(Nucl.)j(Phys.)d fg(A565)g fm(\(1993\))i(158.)-47 1254 y([IV])127 b(G.)16 b(Audi,)g(A.H.)e(W)l(apstra)k(and)f(M.)e(Dedieu,)h fn(Nucl.)j(Phys.)d fg(A565)g fm(\(1993\))i(193.)-47 1320 y([NDS])81 b fn(Nucle)n(ar)18 b(Data)f(She)n(ets)p fm(.)-47 1385 y([53Am08])24 b(D.P)l(.)16 b(Ames)f(et)h(al.,)g fn(Phys.)h(R)n(ev.)f fg(91)h fm(\(1953\))g(68.)-47 1451 y([59T)l(o)o(wn])25 b(C.W.)15 b(T)l(o)o(wnley)i (et)f(al.,)g fn(Bul)r(l.)j(A)o(m.)f(Phys.)f(So)n(c.)f fg(4)g fm(\(1959\))i(366.)-47 1517 y([69Ph01])26 b(M.E.)15 b(Phelps)i(and)g(D.G.)f (Saran)o(tes)h fn(Nucl.)h(Phys.)e fg(A135)h fm(\(1969\))g(116.)-47 1583 y([73Ha11])25 b(J.K.)15 b(Halbig)j(et)e(al.,)g fn(Nucl.)j(Phys.)c fg(A203)i fm(\(1973\))h(532.)-47 1649 y([74An23])24 b(N.M.)15 b(An)o(tonev)m(a)h(et)g(al.,)g fn(Iz.)h(A)o(k.)h(Nauk.)g(SSSR,)g(ser.)g(Fiz.) e fg(38)g fm(\(1974\))i(1748.)-47 1714 y([74Ia01])44 b(R.)15 b(Ia\014gliola,)j(S.C.)e(Gujrathi,)g(B.L.)f(T)l(racy)h(and)g(J.K.P)l(.)f (Lee,)g fn(Can.)i(J.)g(Phys.)e fg(52)h fm(\(1974\))h(96.)-47 1780 y([75Sm02])25 b(L.G.)16 b(Smith)g(and)h(A.H.)e(W)l(apstra,)h fn(Phys.)h(R)n(ev.)f fg(C11)h fm(\(1975\))h(1392.)-47 1846 y([80De02])27 b(R.)15 b(Dec)o(k)o(er)g(et)h(al.,)g fn(Z.)h(Phys.)f fg(A294)h fm(\(1980\))h(35.)-47 1912 y([83Ia02])44 b(R.)15 b(Ia\014gliola,)k(M.)d(Chatterjee,)f(H.)g(Dautet,)i(J.K.P)l(.)e(Lee,)g fn(J.)i(Chem.)f fg(61)h fm(\(1983\))g(694.)-47 1977 y([89Al33])36 b(G.D.)16 b(Alkhazo)o(v)g(et)g(al.,)g fn(Iz.)h(A)o(k.)h(Nauk.)g(SSSR,)g(ser.) f(Fiz.)f fg(53)g fm(\(1989\))i(2089.)-47 2043 y([93Borc])34 b(C.)16 b(Borcea)g(and)h(G.)f(Audi,)g fn(R)n(ev.)h(R)n(oum.)f(Phys.)g fg(38)g fm(\(1993\))i(455.)-47 2109 y([93Kryg])27 b(R.A.)15 b(Kryger)g(et)h(al.,)h fn(Phys.)g(R)n(ev.)f fg(C47)g fm(\(1993\))i(2439.)-47 2175 y([94DiFi])39 b(F.)15 b(DiFilipp)q(o)20 b(et)c(al.,)g(Pro)q(c.)g (ICAP-14,)h(Boulder,)f(1994,)h(p.149)g(and)g(priv)m(ate)g(comm.)-47 2240 y([94Hart])35 b(H.)15 b(Hartmann,)h(Th.-Mainz,)g(1994.)-47 2306 y([94Jurn])36 b(E.T.)16 b(Jurney)f(et)h(al.,)h(Priv)m(ate)g(comm)o (unication)g(to)f(A.H.)f(W)l(apstra,)i(June)f(1994.)-47 2372 y([94Kuma])24 b(V.R.)15 b(Kumar)h(et)g(al.,)g fn(J.)h(Phys.)g(G:)g(Nucl.)i (Phys.)d fg(20)g fm(\(1994\))i(441.)-47 2438 y([94Laza])34 b(Y)l(u.A.)14 b(Lazarev,)i(et)g(al.,)h fn(Phys.)f(R)n(ev.)i(L)n(ett.)e fg(73)g fm(\(1994\))i(624.)-47 2504 y([94Y)l(o01])29 b(B.M.)14 b(Y)l(oung)j(et)f(al.,)g fn(Phys.)h(R)n(ev.)f fg(C49)h fm(\(1994\))h(279.)-47 2569 y([95Bohl])35 b(H.G.)15 b(Bohlen,)h(Priv)m(ate)h(comm)o(unication)g(to)g (G.)f(Audi,)g(Ma)o(y)g(1995.)-47 2635 y([95Boll])49 b(G.)16 b(Bollen)h(et)f(al.,)g fn(Nucl.)j(Phys.)c fg(A)i fm(to)g(b)q(e)f(submitted.) -47 2701 y([95Bren])31 b(D.S.)15 b(Brenner,)g(N.V.)g(Zam\014r)h(and)h(R.F.)e (Casten,)h fn(Phys.)h(R)n(ev.)f fg(C50)h fm(\(1995\))h(490.)-47 2767 y([95Char])29 b(M.)15 b(Chartier)i(et)f(al.,)h(presen)o(ted)e(at)i(this) g(conference)e(\(ENAM'95,)g(Arles,)h(June)g(1995\).)-47 2832 y([95Da)o(vi])35 b(C.N.)15 b(Da)o(vids)i(et)f(al.,)g(presen)o(ted)g(at)g (this)h(conference)e(\(ENAM'95,)h(Arles,)f(June)i(1995\).)-47 2898 y([95Ghio])32 b(A.)15 b(Ghiorso,)j(et)e(al.,)g fn(Nucl.)j(Phys.)c fg(A583)i fm(\(1995\))h(861c.)-47 2964 y([95Grom])24 b(K.Y.)15 b(Gromo)o(v)h(et)g(al.,)h(Priv)m(ate)g(comm)o(unication)g(to)f(G.)g(Audi,)h (April)g(1995.)p eop %%Page: 11 11 bop -47 30 a fm([95Hans])27 b(P)l(.G.)15 b(Hansen,)h(Pro)q(c.)h(Niigata)h (Conference,)d(No)o(v)o(em)o(b)q(er)f(1994,)k(in)f(press.)-47 96 y([95Hart])35 b(H.)15 b(Hartmann)h(et)g(al.,)h fn(Nucl.)h(Phys.)e fg(A)h fm(to)f(b)q(e)h(submitted.)-47 162 y([95Ho.1])35 b(S.)16 b(Hofmann,)g(et)f(al.,)i fn(Z.)g(Phys.)f fg(A350)g fm(\(1995\))i(277.)-47 229 y([95Ho.2])35 b(S.)16 b(Hofmann,)g(et)f(al.,)i fn(Z.)g(Phys.)f fg(A350)g fm(\(1995\))i(281.)-47 295 y([95Ho.A])23 b(S.)16 b(Hofmann,)g(et)g(al.,)g(GSI-Nac)o(hr.)f(F)l(ebruary)h(1995.)-47 361 y([95Lepi])42 b(A.)15 b(L)o(\023)-23 b(epine)17 b(et)f(al.,)g(presen)o (ted)g(at)g(this)h(conference)e(\(ENAM'95,)g(Arles,)h(June)g(1995\).)-47 427 y([95Ogan])25 b(Y)l(u.)15 b(Ts.)h(Oganessian,)i(presen)o(ted)e(at)g(this) h(conference)f(\(ENAM'95,)f(Arles,)g(June)i(1995\).)-47 494 y([95Raim])24 b(H.)16 b(Raim)o(bault-Hartmann)i(et)e(al.,)g(presen)o(ted)f (at)i(this)g(conference)e(\(ENAM'95,)g(June)h(95\).)-47 560 y([95Rous])28 b(B.)15 b(Roussi)o(\022)-23 b(ere)17 b(et)f(al.,)g fn(Z.)i(Phys.)d fg(A351)i fm(\(1995\))h(127.)-47 626 y([95Szer])44 b(J.)16 b(Szeryp)q(o)g(et)g(al.,)g fn(Nucl.)j(Phys.)c fg(584)i fm(\(1995\))g(221.)-47 692 y([95W)l(aps])25 b(A.H.)14 b(W)l(apstra,)j(to)g(b) q(e)f(published.)-47 759 y([95Zins])45 b(M.)15 b(Zinser)i(et)f(al.,)g (Preprin)o(t)g(GSI-95-03.)p eop %%Trailer end userdict /end-hook known{end-hook}if %%EOF

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